High-fidelity spherical cholesteric liquid crystal Bragg reflectors generating unclonable patterns for secure authentication

Author(s)
Yong Geng, JungHyun Noh, Irena Drevensek-Olenik, Romano Rupp, Gabriele Lenzini, Jan P. F. Lagerwall
Abstract

Monodisperse cholesteric liquid crystal microspheres exhibit spherically symmetric Bragg reflection, generating, via photonic cross communication, dynamically tuneable multi-coloured patterns. These patterns, uniquely defined by the particular sphere arrangement, could render cholesteric microspheres very useful in countless security applications, as tags to identify and authenticate their carriers, mainly physical objects or persons. However, the optical quality of the cholesteric droplets studied so far is unsatisfactory, especially after polymerisation, a step required for obtaining durable samples that can be used for object identification. We show that a transition from droplets to shells solves all key problems, giving rise to sharp patterns and excellent optical quality even after polymerisation, the polymerised shells sustaining considerable mechanical deformation. Moreover, we demonstrate that, counter to prior expectation, cross communication takes place even between non-identical shells. This opens additional communication channels that add significantly to the complexity and unique character of the generated patterns.

Organisation(s)
Physics of Functional Materials
External organisation(s)
University of Luxembourg, University of Ljubljana, Jožef Stefan Institute (IJS)
Journal
Scientific Reports
Volume
6
No. of pages
9
ISSN
2045-2322
DOI
https://doi.org/10.1038/srep26840
Publication date
05-2016
Peer reviewed
Yes
Austrian Fields of Science 2012
103021 Optics
Keywords
Portal url
https://ucris.univie.ac.at/portal/en/publications/highfidelity-spherical-cholesteric-liquid-crystal-bragg-reflectors-generating-unclonable-patterns-for-secure-authentication(e7a9595f-2006-4274-a2c8-bfa12316966e).html